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Abstract The emergence of atomically thin van der Waals magnets provides a new platform for the studies of two-dimensional magnetism and its applications. However, the widely used measurement methods in recent studies cannot provide quantitative information of the magnetization nor achieve nanoscale spatial resolution. These capabilities are essential to explore the rich properties of magnetic domains and spin textures. Here, we employ cryogenic scanning magnetometry using a single-electron spin of a nitrogen-vacancy center in a diamond probe to unambiguously prove the existence of magnetic domains and study their dynamics in atomically thin CrBr 3 . By controlling the magnetic domain evolution as a function of magnetic field, we find that the pinning effect is a dominant coercivity mechanism and determine the magnetization of a CrBr 3 bilayer to be about 26 Bohr magnetons per square nanometer. The high spatial resolution of this technique enables imaging of magnetic domains and allows to locate the sites of defects that pin the domain walls and nucleate the reverse domains. Our work highlights scanning nitrogen-vacancy center magnetometry as a quantitative probe to explore nanoscale features in two-dimensional magnets. 

Moiré superlattices of twisted nonmagnetic two-dimensional (2D) materials are highly controllable platforms for the engineering of exotic correlated and topological states. Here, we report emerging magnetic textures in small-angle twisted 2D magnet chromium triiodide (CrI 3 ). Using single-spin quantum magnetometry, we directly visualized nanoscale magnetic domains and periodic patterns, a signature of moiré magnetism, and measured domain size and magnetization. In twisted bilayer CrI 3 , we observed the coexistence of antiferromagnetic (AFM) and ferromagnetic (FM) domains with disorder-like spatial patterns. In twisted double-trilayer CrI 3 , AFM and FM domains with periodic patterns appear, which is in good agreement with the calculated spatial magnetic structures that arise from the local stacking-dependent interlayer exchange interactions in CrI 3 moiré superlattices. Our results highlight magnetic moiré superlattices as a platform for exploring nanomagnetism. 

Iron‐rich olivine is mechanically weaker than olivine of mantle composition, ca. Fo₉₀, and thus is more amenable to study under a wide range of laboratory conditions. To investigate the effects of iron content on deformation‐produced crystallographic preferred orientation (CPO) and grain size, we analyzed the microstructures of olivine samples with compositions of Fo₇₀, Fo₅₀, and Fo₀that were deformed in torsion under either anhydrous or hydrous conditions at 300 MPa. Electron backscatter diffraction (EBSD) observations reveal a transition in CPO from D‐type fabric, induced by dislocation glide on both the (010)[100] and the (001)[100] slip systems, at low strains, to A‐type fabric, caused by dislocation glide on the (010)[100] slip system, at high strains for all of our samples, independent of iron content and hydrous/anhydrous conditions. A similar evolution of fabric with increasing strain is also reported to occur for Fo₉₀. Radial seismic anisotropy increases with increasing strain, reaching a maximum value of ∼1.15 at a shear strain of ∼3.5 for each sample, demonstrating that the seismic anisotropy of naturally deformed olivine‐rich rocks can be well approximated by that of iron‐rich olivine. Based on EBSD observations, we derived a piezometer for which recrystallized grain size decreases inversely with stress to the ∼1.2 power. Also, recrystallized grain size increases with increasing iron content. Our experimental results contribute to understanding the microstructural evolution in the mantle of not only Earth but also Mars, where the iron content in olivine is higher.